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基于单宁酸负载的自预警-自修复双重功能防腐涂层

马菱薇 杨雪婷 郑凯宁 王金科 王悦 杨昊

马菱薇, 杨雪婷, 郑凯宁, 王金科, 王悦, 杨昊. 基于单宁酸负载的自预警-自修复双重功能防腐涂层[J]. 材料开发与应用, 2024, 39(2): 95-105.
引用本文: 马菱薇, 杨雪婷, 郑凯宁, 王金科, 王悦, 杨昊. 基于单宁酸负载的自预警-自修复双重功能防腐涂层[J]. 材料开发与应用, 2024, 39(2): 95-105.
MA Lingwei, YANG Xueting, ZHENG Kaining, WANG Jinke, WANG Yue, YANG Hao. Self-Reporting and Self-Healing Dual Functional Anticorrosive Coating based on Tannic Acid Additives[J]. Development and Application of Materials, 2024, 39(2): 95-105.
Citation: MA Lingwei, YANG Xueting, ZHENG Kaining, WANG Jinke, WANG Yue, YANG Hao. Self-Reporting and Self-Healing Dual Functional Anticorrosive Coating based on Tannic Acid Additives[J]. Development and Application of Materials, 2024, 39(2): 95-105.

基于单宁酸负载的自预警-自修复双重功能防腐涂层

详细信息
    作者简介:

    马菱薇,女,1990年生,副研究员,硕士生导师,主要研究方向为智能耐蚀材料与表面技术。E-mail:mlw1215@[KG-*3]ustb.edu.cn

  • 中图分类号: TG178

Self-Reporting and Self-Healing Dual Functional Anticorrosive Coating based on Tannic Acid Additives

  • 摘要: 通过一步合成法制备了负载单宁酸(TA)的显色、缓蚀双功能介孔二氧化硅纳米填料(TA-MSNs),将其掺杂到环氧涂层中,探究涂层的自预警和自修复性能。首先对TA的显色性能及缓蚀性能进行了表征,接着对TA-MSNs纳米填料的形貌结构以及TA的释放行为规律进行了探究,并综合分析纳米填料添加量对涂层自预警及自修复性能的影响规律。盐雾实验结果表明,涂层的自预警效果与填料含量呈正相关,5 %(w)以上的TA-MSNs添加量可赋予涂层明显的显色性能。电化学阻抗谱和表面分析结果表明,TA-MSNs在涂层中的含量为5 %时,破损涂层的低频阻抗模值比纯环氧破损涂层高出2个数量级。当涂层破损时,涂层中释放的TA分子能够与钢铁腐蚀形成的Fe3+发生络合,产生蓝黑色预警金属腐蚀,同时络合物可形成金属表面保护膜层,抑制了腐蚀反应的进一步发展。综上,添加5 % TA-MSNs的环氧涂层具有优异的自预警和自修复效果。

     

  • [1] LI X G, ZHANG D W, LIU Z Y, et al. Materials science:share corrosion data[J]. Nature, 2015, 527:441-442.
    [2] 冷文俊, 崔中雨, 王昕, 等. 低合金高强钢极地环境加速腐蚀试验谱编制与研究[J]. 材料开发与应用, 2023, 38(3):31-36.
    [3] 聂淑坤, 许凤玲, 刘钊慧, 等. 硫酸盐还原菌对船体低合金裸钢腐蚀行为的影响[J]. 材料开发与应用, 2023, 38(1):29-41.
    [4] JING Y, MENG F D, WANG F H, et al. Design of an anticorrosion/bactericidal dual functional organic coating based on the slippery liquid-infused porous surface[J]. Applied Surface Science, 2023, 639:158214.
    [5] DING C D, TAI Y, WANG D, et al. Superhydrophobic composite coating with active corrosion resistance for AZ31B magnesium alloy protection[J]. Chemical Engineering Journal, 2019, 357:518-532.
    [6] 祁伟健, 谢延凯, 汤一尧, 等. 典型有机防腐涂层研究进展[J]. 甘肃科技, 2023, 39(9):111-115.
    [7] LIU C B, CHENG L, QIAN B, et al. Corrosion self-warning and repair tracking of polymeric coatings based on stimulus responsive nanosensors[J]. Nan-oscale, 2022, 14(23):8429-8440.
    [8] MA L W, REN C H, WANG J K, et al. Self-reporting coatings for autonomous detection of coating damage and metal corrosion:a review[J]. Chemical Engineering Journal, 2021, 421:127854.
    [9] 周少魁, 郭宏磊, 顾林. 荧光涂层的设计、制备与应用研究进展[J]. 表面技术, 2021, 50(11):30-48.
    [10] WANG Y, WANG J K, HUANG L Y, et al. Photothermally activated self-healing coatings for corrosion protection:a review[J]. Progress in Organic Coa-tings, 2023, 185:107886.
    [11] ZHANG F, JU P F, PAN M Q, et al. Self-healing mechanisms in smart protective coatings:a review[J]. Corrosion, 2018, 144:74-88.
    [12] 许超, 肖调兵, 乔泽, 等. 智能防腐涂层的研究进展及其在国内核电领域的应用前景[J]. 腐蚀与防护, 2023, 44(4):65-71.
    [13] Y1 LD1 Z M, SAHINER N. Tannic acid for simple and highly selective visual detection of iron (II) and (III) ions from different aqueous environments[J]. Water, Air, & Soil Pollution, 2021, 232(5):201.
    [14] WANG J K, TAN W M, YANG H, et al. Towards weathering and corrosion resistant, self-warning and self-healing epoxy coatings with tannic acid loaded nanocontainers[J]. NPJ Materials Degradation, 2023, 7:39.
    [15] DEMENT'EVA O V.Mesoporous silica container particles:new approaches and new opportunities[J]. Colloid Journal, 2020, 82(5):479-501.
    [16] YANG H, LIAO S J, HUANG C, et al. Facile one-pot approach to the synthesis of spherical mesoporous silica nanoflowers with hierarchical pore structure[J]. Applied Surface Science, 2014, 314:7-14.
    [17] QIAN B, ZHENG Z, MICHAILIDS M, et al. Mussel-inspired self-healing coatings based on polydopamine-coated nanocontainers for corrosion protection[J]. ACS Applied Materials & Interfaces, 2019, 11(10):10283-10291.
    [18] 周游, 周帅, 周江鸿, 等. 硅烷化氧化石墨烯/有机硅复合涂层的制备及性能[J]. 电镀与涂饰, 2023, 42(16):63-70.
    [19] RAMEZANZADEH B, NIROUMANDRAD S, AHMA-DI A, et al. Enhancement of barrier and corrosion protection performance of an epoxy coating through wet transfer of amino functionalized graphene oxide[J]. Corrosion, 2016, 103:283-304.
    [20] MA L W, WANG J K, ZHANG D W, et al. Dual-action self-healing protective coatings with pho-tothermal responsive corrosion inhibitor nanocontainers[J]. Che-mical Engineering Journal, 2021, 404:127118.
    [21] 赵芳, 许立坤, 李相波. 铝粉含量对锌铝涂层微观形貌和耐蚀性的影响[J]. 材料开发与应用, 2012, 27(3):46-50.
    [22] 陶乃旺, 曾登峰, 王佳妮. 电解海水对环氧涂层防腐蚀性能的影响研究[J]. 材料开发与应用, 2021, 36(5):38-44.
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出版历程
  • 收稿日期:  2023-10-25
  • 网络出版日期:  2024-05-09

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